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학술논문Bulletin of the Korean Chemical Society2022.01 발행

Method development of phenolic acid profiling analysis as tert-butyldimethylsilyl derivative by gas chromatographytandem mass spectrometry

Method development of phenolic acid profiling analysis as tert-butyldimethylsilyl derivative by gas chromatographytandem mass spectrometry

Kim Youngbae(College of Pharmacy Sunchon National University Suncheon Republic of Korea); Seo Chan(College of Pharmacy Sunchon National University Suncheon Republic of Korea); Lee Hyeon‐Seong(College of Pharmacy Sunchon National University Suncheon Republic of KoreaNatural Product Informatics Research Center Gangneung Institute of Natural Products, Korea Institute of Science and Technology Gangwon‐do Republic of Korea); Ji Moongi(College of Pharmacy Sunchon National University Suncheon Republic of Korea); Oh Songjin(College of Pharmacy Sunchon National University Suncheon Republic of Korea); Choi Byeong‐Chan(College of Pharmacy Sunchon National University Suncheon Republic of Korea); Kim Doo‐Young(College of Pharmacy Sunchon National University Suncheon Republic of Korea); Park Kyung‐Wuk(Suncheon Research Center for Natural Medicines Suncheon South Korea); 박준성(Department of Engineering Chemistry College of Engineering, Chungbuk National University Republic of Korea); Paik Man‐Jeong(College of Pharmacy Sunchon National University Suncheon Republic of Korea)

43권 1호, 88~92쪽

초록

An efficient gas chromatography-tandem mass spectrometry-based method using tert-butyldimethylsilyl derivative was developed for the simultaneous analysis of 10 phenolic acids. Under optimal conditions, linearity in the range of 2–100 ng/ml exhibited correlation coefficient (r) of ≥0.999. Repeatability showed low relative standard deviation of <16.7%, and accuracy (% relative error) varied from 9.8 to 3.4. New mass spectra data sets of 10 phenolic acids were constructed in multiple reaction monitoring mode. When applied to Orostachys japonica (Maxim.) A. Berger, the 10 phenolic acids of salicylic, 4-hydroxybenzoic, vanillic, m-coumaric, syringic, p-coumaric, protocatechuic, ferulic, gallic, and caffeic acids were positively identified. We believe that the devised method will be found useful for profiling phenolic acids in various plant samples.

Abstract

An efficient gas chromatography-tandem mass spectrometry-based method using tert-butyldimethylsilyl derivative was developed for the simultaneous analysis of 10 phenolic acids. Under optimal conditions, linearity in the range of 2–100 ng/ml exhibited correlation coefficient (r) of ≥0.999. Repeatability showed low relative standard deviation of <16.7%, and accuracy (% relative error) varied from 9.8 to 3.4. New mass spectra data sets of 10 phenolic acids were constructed in multiple reaction monitoring mode. When applied to Orostachys japonica (Maxim.) A. Berger, the 10 phenolic acids of salicylic, 4-hydroxybenzoic, vanillic, m-coumaric, syringic, p-coumaric, protocatechuic, ferulic, gallic, and caffeic acids were positively identified. We believe that the devised method will be found useful for profiling phenolic acids in various plant samples.

발행기관:
대한화학회
DOI:
http://dx.doi.org/10.1002/bkcs.12423
분류:
화학

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Method development of phenolic acid profiling analysis as tert-butyldimethylsilyl derivative by gas chromatographytandem mass spectrometry | Bulletin of the Korean Chemical Society 2022 | AskLaw | 애스크로 AI